
本教材共分为9章,系统介绍了单光子吸收理论,单光子诱导电子空穴相关性,在生物、材料、SERS中的单光子过程,双光子吸收理论,非线性极化率理论,双光子诱导电子空穴相关性和双光子荧光分子应用等内容。本书内容深入浅出,通俗易懂。
本教材适用于物理学、光学、化学、材料学等专业
科研院所和高校的研究人员、研究生及高年级本科生使用。
Sun Mengtaoobtained his Ph.D. in 2003 from the State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences (CAS). From 2003 to 2006, he worked as a postdoc at the Department of Chemical Physics, Lund University. Since 2006, as an associate professor, he has worked at the Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences(CAS). In 2016, he became a full professor in University of Science and Technology Beijing, China. His current research interests focus on oneand twophoton absorptions in organic molecules, twodimensional (2D) materials and plasmonics, as well as the excitonplasmon coupling interaction for surface catalytic reaction. He has published more than 150 papers, including 10 invited review papers, three books and three book chapters in English, and citations are about 5000 times. Researcher ID: B11312008. In 2016, He was awarded the second prize of Science and Technology in Liaoning province.
Li Yuanzuoearned his Ph.D. in the School of Physics, Dalian University of Technology (DLUT) in 2011. He became an associate professor in Northeast Forestry University in 2014. His current research interests include: experiment and first principle calculation on solar cells, excited state dynamics, energy conversion and nanomaterials. He has published more than 60 scientific publications, reviews and book chapters in the field of excited state properties of organic systems.
CHAPTER 1OnePhoton Absorption Theory
References
CHAPTER 2Charge Transfer and ElectronHole Coherence in OPA
References
CHAPTER 3Application of OPA
3.1Biology
3.1.1Retinal proteins (rhodopsins)
3.1.2Green fluorescent protein
3.2Enenrgy materials
3.2.1Quinoidal charge delocalization in polyp
phenylene cation radical
3.2.2Neutral and charged πdimeric quinquethiophenes
3.2.3Surfaceenhanced resonance Raman scattering
3.2.4Near and deepUV resonance Raman spectroscopy of
pyrazineAl4 complex and Al3pyrazineAl3 junction
References
CHAPTER 4TwoPhoton Absorption
4.1TPA section
4.2Experimental methods and TPA materials
References
CHAPTER 5Polarizabilities in Absorption Processes
References
CHAPTER 6Charge Transfer and ElectronHole Coherence in TPA
6.13D cube and 2D site representations for TPA
6.2Quantum chemical calculations
6.3
Visualizations of transition dipoles, charge transfer and
electronhole coherence on electronic state transitions
between excited states for TPA
6.4Photoexcitation mechanisms of centrosymmetric and
asymmetric fluorine derivatives in TPA
References
CHAPTER 7Application of TPA
7.1Twophoton photophysical properties of tri9anthrylborane
7.2Spectroscopic and theoretical studies on the photophysical
properties of dichlorotriazine derivatives
References
CHAPTER 8Modeling Examples of Photon Absorptions and
Nonlinear Properties in ProAromatic Chromophores
References
CHAPTER 9Modeling Examples of Simulated Polymethine Dyes
for AllOptical Witching
Summary
References
Acknowledgements
本教材适用于物理、光学、化学和材料学等专业科研院所和高校的研究人员、研究生及高年级本科生使用。
本书作者孙萌涛,北京科技大学教授,博导,多本教材适用于物理、光学、化学和材料学等专业科研院所和高校的研究人员、研究生及高年级本科生使用。年从事相关专业研究工作。